Population Redistribution in a Continuously Driven Λ-Type Semiconductor Quantum Dot: Roles of Relaxation-Path Asymmetry And Off-Resonant Coupling

Arik Ramadhan, Bintoro Siswo Nugroho, Asifa Asri, Azrul Azwar, Yudha Arman

Abstract

Semiconductor quantum dots (SQDs) exhibit optical responses that are strongly influenced by their internal level structure, relaxation pathways, and excitation intensity. This study investigates the time- and intensity-dependent population dynamics of a continuously driven single Λ-type three-level SQD using the density-matrix formalism within the rotating-wave approximation. Dissipative processes are incorporated through Lindblad-type relaxation terms, while the transient and stationary responses are obtained, respectively, by numerical time integration and steady-state solution of the density-matrix equations. Special attention is given to the relaxation channel γ32 and the off-resonant transition dipole moment μ32. The results show that γ32 primarily controls the transient redistribution route and the timescale required to reach the stationary regime, whereas the early oscillatory behavior remains dominated by the resonantly driven |1⟩ ↔|3⟩ transition. In the steady-state regime, γ32 mainly determines how population leaving the upper state is partitioned between the two lower states, while μ32 governs how readily the off-resonant |2⟩ ↔|3⟩ branch becomes active as the driving intensity increases. Consequently, the crossover from predominantly resonant two-level-like behavior to genuine three-level population redistribution is controlled by the combined action of relaxation-path asymmetry and off-resonant coupling strength. These findings provide a clearer mechanism-based interpretation of driven population redistribution in effective multilevel SQD systems.

Keywords

continuous-wave excitation; density-matrix formalism; population dynamics; semiconductor quantum dots; Λ-type three-level system

References

Boos, K., Kim, S. K., Bracht, T., Sbresny, F., Kaspari, J. M., Cygorek, M., Riedl, H., Bopp, F. W., Rauhaus, W., Calcagno, C., Finley, J. J., Reiter, D. E., & Müller, K. (2024). Signatures of Dynamically Dressed States. Physical Review Letters, 132(5), 53602. https://doi.org/10.1103/PhysRevLett.132.053602

Feng, D., Zhang, G., & Li, Y. (2024). Semiconductor Quantum Dots: Synthesis, Properties and Applications. In Nanomaterials (Vol. 14, Issue 22, p. 1825). https://doi.org/10.3390/nano14221825

Grisard, S., Rose, H., Trifonov, A. V, Reichhardt, R., Reiter, D. E., Reichelt, M., Schneider, C., Kamp, M., Höfling, S., Bayer, M., Meier, T., & Akimov, I. A. (2022). Multiple Rabi rotations of trions in InGaAs quantum dots observed by photon echo spectroscopy with spatially shaped laser pulses. Physical Review B, 106(20), 205408. https://doi.org/10.1103/PhysRevB.106.205408

Heindel, T., Kim, J.-H., Gregersen, N., Rastelli, A., & Reitzenstein, S. (2023). Quantum dots for photonic quantum information technology. Advances in Optics and Photonics, 15(3), 613–738. https://doi.org/10.1364/AOP.490091

Hu, X., Zhang, Y., Guzun, D., Ware, M. E., Mazur, Y. I., Lienau, C., & Salamo, G. J. (2020). Photoluminescence of InAs/GaAs quantum dots under direct two-photon excitation. Scientific Reports, 10(1), 10930. https://doi.org/10.1038/s41598-020-67961-z

Khanonkin, I., Bauer, S., Eyal, O., Reithmaier, J. P., & Eisenstein, G. (2022). Steering coherence in quantum dots by carriers injection via tunneling. Nanophotonics, 11(15), 3457–3463. https://doi.org/https://doi.org/10.1515/nanoph-2022-0184

Kosarev, A. N., Trifonov, A. V, Yugova, I. A., Yanibekov, I. I., Poltavtsev, S. V, Kamenskii, A. N., Scholz, S. E., Sgroi, C. A., Ludwig, A., Wieck, A. D., Yakovlev, D. R., Bayer, M., & Akimov, I. A. (2022). Extending the time of coherent optical response in ensemble of singly-charged InGaAs quantum dots. Communications Physics, 5(1), 144. https://doi.org/10.1038/s42005-022-00922-2

Löbl, M. C., Scholz, S., Söllner, I., Ritzmann, J., Denneulin, T., Kovács, A., Kardynał, B. E., Wieck, A. D., Ludwig, A., & Warburton, R. J. (2019). Excitons in InGaAs quantum dots without electron wetting layer states. Communications Physics, 2(1), 93. https://doi.org/10.1038/s42005-019-0194-9

Lu, X., Huang, D., & Fan, S. (2021). Effect of Coulomb interaction on the transient optical response of electrons in field-coupled quantum dots. Physical Review A, 103(4), 43504. https://doi.org/10.1103/PhysRevA.103.043504

Man, M. T., & Lee, H. S. (2019). Clarifying photoluminescence decay dynamics of self-assembled quantum dots. Scientific Reports, 9(1), 4613. https://doi.org/10.1038/s41598-019-41075-7

Manson, R., Roy-Choudhury, K., & Hughes, S. (2016). Polaron master equation theory of pulse-driven phonon-assisted population inversion and single-photon emission from quantum-dot excitons. Physical Review B, 93(15), 155423. https://doi.org/10.1103/PhysRevB.93.155423

Meng, L., Xu, Q., Zhang, J., & Wang, X. (2024). Colloidal quantum dot materials for next-generation near-infrared optoelectronics. Chemical Communications, 60(9), 1072–1088. https://doi.org/10.1039/D3CC04315K

Moody, G., & Cundiff, S. T. (2017). Advances in multi-dimensional coherent spectroscopy of semiconductor nanostructures. Advances in Physics: X, 2(3), 641–674. https://doi.org/10.1080/23746149.2017.1346482

Nugroho, B. S., Iskandar, A. A., Malyshev, V. A., & Knoester, J. (2020). Plasmon-assisted two-photon absorption in a semiconductor quantum dot-metallic nanoshell composite. Physical Review B, 102(4), 1–8. https://doi.org/10.1103/PhysRevB.102.045405

Paspalakis, E., Smponias, A., & Stefanatos, D. (2021). Coherent preparation of the biexciton state in a semiconductor quantum dot coupled to a metallic nanoparticle. Journal of Applied Physics, 129(22), 223104. https://doi.org/10.1063/5.0053859

Poltavtsev, S. V, Reichelt, M., Akimov, I. A., Karczewski, G., Wiater, M., Wojtowicz, T., Yakovlev, D. R., Meier, T., & Bayer, M. (2017). Damping of Rabi oscillations in intensity-dependent photon echoes from exciton complexes in a CdTe/(Cd,Mg)Te single quantum well. Physical Review B, 96(7), 75306. https://doi.org/10.1103/PhysRevB.96.075306

Ryzhov, I. V., Malikov, R. F., Malyshev, A. V., & Malyshev, V. A. (2019). Nonlinear optical response of a two-dimensional quantum-dot supercrystal: Emerging multistability, periodic and aperiodic self-oscillations, chaos, and transient chaos. Physical Review A, 100(3). https://doi.org/10.1103/PhysRevA.100.033820

Ryzhov, I. V., Malikov, R. F., Malyshev, A. V., & Malyshev, V. A. (2021). Quantum metasurfaces of arrays of Λ-emitters for photonic nano-devices. Journal of Optics (United Kingdom), 23(11), 1–14. https://doi.org/10.1088/2040-8986/ac2788

Stachurski, J., Tamariz, S., Callsen, G., Butté, R., & Grandjean, N. (2022). Single photon emission and recombination dynamics in self-assembled GaN/AlN quantum dots. Light: Science & Applications, 11(1), 114. https://doi.org/10.1038/s41377-022-00799-4

Tohari, M. M., Alqahtani, M. M., & Lyras, A. (2020). Optical Multistability in the Metal Nanoparticle–Graphene Nanodisk–Quantum Dot Hybrid Systems. In Nanomaterials (Vol. 10, Issue 9, p. 1687). https://doi.org/10.3390/nano10091687

Veisi, M., Kazemi, S. H., & Mahmoudi, M. (2020). Tunneling-induced optical limiting in quantum dot molecules. Scientific Reports, 10(1), 16304. https://doi.org/10.1038/s41598-020-73343-2

Zhou, X., Zhai, L., & Liu, J. (2023). Epitaxial quantum dots: a semiconductor launchpad for photonic quantum technologies. Photonics Insights, 1(2), R07–R07. https://doi.org/http://dx.doi.org/10.3788/PI.2022.R07

Refbacks

  • There are currently no refbacks.